Phantom helix states in Heisenberg quantum magnets

Jepsen, P.N., Lee, Y.K., Lin, H. et al. Long-lived phantom helix states in Heisenberg quantum magnets. Nat. Phys. 18, 899–904 (2022).

You can find an article on summarizing our work here.

Quantum magnetism underlies many of the technologies we use today, including memory storage devices, and is thus of fundamental interest. To model quantum magnetism, one can depict each elementary particle as carrying a spin which can point in different directions. In this context, two nearby spins can exchange their relative orientations via an intermediate state with both particles in the same place. 

This idea is captured by a simple textbook model called the Heisenberg spin model, which can be realized in one dimension (i.e., a chain) in our experimental platform using ultracold atoms. 

Generically if we prepare a simple pattern of spins, say all spins aligned, then over time the pattern will thermalize to a random mixture of spins pointing in all different directions and lose the information about the initial state. These phantom helix states are special because they are protected against thermalization.


The experimental observation of long-lived phantom helix states in Heisenberg quantum magnets

In non-integrable systems (e.g. in higher dimensions or with long-range interactions), phantom helix states are actually quantum many-body scars, which are under intense investigation by the quantum community. The XXZ Heisenberg model is one of the simplest many-body systems that can be realized that can also support scars.

Spin Transport in a Tunable Heisenberg Model

Jepsen, P.N., Amato-Grill, J., Dimitrova, I. et al. Spin transport in a tunable Heisenberg model realized with ultracold atoms. Nature 588, 403–407 (2020).

Simple spin physics captures the properties of many systems such as magnetic materials, high-Tc superconductors, systems with gauge fields, and more. Creating a versatile platform to study and compare these models has been a long-standing goal in the field of ultracold atoms. To that end, our lab has recently implemented the Heisenberg XXZ model with tunable interactions (see above).

Nearest-neighbor couplings are mediated by superexchange (see below). We control the ratio between the transverse coupling (Jxy) and longitudinal coupling (Jz), the "anisotropy," by tuning an applied magnetic field through Feshbach resonances between the two lowest hyperfine states at high magnetic fields. Thus, we can explore the dynamics of spin transport throughout a broad range of anisotropies.

We prepare a far out-of-equilibirum initial state, a "spin helix." and find that the characteristic time for spin transport scales as a power-law with the inverse of the wave vector Q = (2π / λ) of the helix. In other words, τ ~ Q. While scalings of ballistic-like transport (α = 1) and diffusive-like transport (α = 2) had been predicted by theory, we unexpectedly discovered that the exponent α also varies smoothly with anisotropy between 1 and 2 (super-diffusive transport), and even above 2 (sub-diffusive transport).


Enhanced Superexchange in a Tilted Lattice

Dimitrova, I., Jepsen, N., Buyskikh, A., Venegas-Gomez, A., Amato-Grill, J., Daley, A., & Ketterle, W. (2020). Enhanced Superexchange in a Tilted Mott Insulator. Phys. Rev. Lett., 124(4), 43204.

When a tilt is added to the Mott insulator, first order tunneling (at t) is suppressed, while second order tunneling (superexchange, at t2/U) persists. This separation between mass and entropy transport (at t) and spin dynamics at t2/U has several new features for studying spin physics. (i) Arbitrary initial density distributions can be used because the tilt can freeze them in. (ii) The Mott insulator - to - superfluid transition can be suppressed, so that spin dynamics can be studied at lower lattice depths, where the dynamics are faster. (iii) The parameters of the spin Hamiltonian can be tuned with the tilt. (iv) Defects, such as holes and doublons, are made immobile by the tilt, enabling the study of pure spin dynamics.

Quantum Magnetism

We use the lowest two hyperfine states of Li 7 at high magnetic field to realize the 2-component Bose-Hubbard model. We are interested in studying phenomena in Quantum Magentism: the ordered phases which arise when the dominant interaction between particles on a lattice is superexchange. In particular, the 2-component Bose Hubbard Hamiltonian can be directly mapped onto the Heisenberg spin Hamilitonan. In the context of the Bose Hubbard model, superexchange is a second order tunneling process, characterized by a matrix element "t2/U." Here "t" is the hopping and "U" is the on-site interaction. The phase diagram of this Hamiltonian includes feromagnetic and anti-ferromagnetic phases aligned either with the quantization axis "z" or with a line in the the "xy"-plane. The main limitations so far for observing the full phase diagram of this model have been the slow rate of the superexchange process compared to the lifetimes of cold atoms in optical lattices and the very low critical temperatures required for superexchange to be the dominant interactions. Li 7 promises to make improvements on both fronts. Its light mass leads to faster tunneling, compared to other atoms, such as Rb, commonly used in Quantum Simulation experiments, so "t2/U" is large. In addition, the critical temperature for magnetic ordering is also on the order of "t2/U," so it can be reached more easily with Li.

Spin 1/2

Starting from an n=1 Mott insulator, we can simulate the s=1/2 Hubbard model. 


Spin 1

Starting from an n=2 Mott insulator, we can simulate the s=1 Hubbard model. 

Interaction Spectroscopy

Amato-Grill, J., Jepsen, N., Dimitrova, I., Lunden, W., & Ketterle, W. (2019). Interaction spectroscopy of a two-component Mott insulator. Physical Review A, 99(3), 1–5.

We would like to realize a Spin 1 model with the lowest two hyperfine states of Li 7 by going into a Mott insulator with two atoms per site. We call the lowest two hyperfine states "a" and "b." 

Interaction spectroscopy relies on the fact that the interactions between two atoms on a site depend on the spin configuration of the two atoms. For example, the interactions between two "a" atoms, Uaa are in principle different from the interactions between an "a" and a "b" atom, Uab. The RF transition frequency between two "a" atoms on a site and an "a" and a "b" atom on a site is shifted from the bare transition between a single "a" and a single "b" atom on a site by the interaction difference Uab-Uaa. We can flip only one of the two atoms per site when the interaction differences are not degenerate, i.e. Uab-Uaa is not equal to Ubb-Uab. If the interaction differences are degenerate, we can drive a transition from "bb" all the way to "aa."

We prepare a Mott insulator of "b" atoms and drive a spin flip transition from "b" to "a." We measure the number of spin flipped atoms (the number of "a" atoms) and we observe two peaks: One corresponding to the transition of the n=1 shell of the Mott insulator at the bare transition frequency, and one of the n=2 shell at a frequency shifted by the interaction difference Uab-Uaa

We use interaction spectroscopy to map out the interaction differences across the Feshbach resonances of Li 7. In addition, we use amplitude modulation spectroscopy to measure the absolute value of the interactions.  

Finally, we find a point at which the interactions are degenerate and drive a full Rabi oscillation between "bb" and "aa"

New Superradiant Regimes in a BEC

We study superradiance with two non-interacting counterpropagating beams along the long axis of a BEC. We find that there are two regimes in which the system behaves qualitatively differently. At low Rayleigh scattering rates, the stimulated emission from the two beams cancel. At large Rayleigh scattering rates, we see evidense of a formation of a different phase. Such a phase has been predicted in  [S. Ostermann, F. Piazza, and H. Ritsch, Phys. Rev. X 6, 021026 (2016)].  It consists of a stationary density modulation and a standing optical wave. See our results here:

Superradiance with a single pump beam: moving density modulation


Two non-interfering pump beams:


Noise in Optical Lattices

We have studied noise and heating in optical lattices extensively. 

Li 7 BEC

Here is a graph showing the cooling steps we take to make a Li 7 BEC. 


CUA Retreat poster (Jan 2017)

CUA Retreat poster (Jan 2016)

NSF visit poster (MIT, April 28, 2014)

Gordon Conference (Newport, June 2013)

DAMOP (June 2012)

Summer School in Granada, Spain (September 2011)